Abstract
We developed a cost-effective method to manufacture high performance-monolithic solid oxide fuel cells using nano-composite electrodes, tape-casting and single-step co-firing. NiO/YSZ-YSZ nano-composite powder comprising nano-sized NiO and YSZ adhered to core YSZ powder was prepared for anode support. LSM/GDC nano-composite cathode fired at 1400 C had a porosity of over 20%, which was much higher than that of conventional LSM-GDC. Furthermore, the area specific resistance of the LSM/GDC cathode was 0.15 Ω cm 2, which was much lower than that of the LSM-GDC and LSM-YSZ mechanically mixed cathodes. Various types of monolithic SOFC unit cells were prepared; one consisting of a NiO-YSZ anode, NiO/YSZ-YSZ anode functional layer, and LSM-GDC cathode had a current density of 0.37 A/cm2 at 0.7 V at 800 C. Optimized monolithic SOFC consisting of NiO/YSZ-YSZ anode and YSZ electrolyte and LSM/GDC cathode had a greatly improved current density of 0.84 A/cm2.
| Original language | English |
|---|---|
| Pages (from-to) | 2313-2319 |
| Number of pages | 7 |
| Journal | International Journal of Hydrogen Energy |
| Volume | 39 |
| Issue number | 5 |
| DOIs | |
| Publication status | Published - 2014 Feb 4 |
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All Science Journal Classification (ASJC) codes
- Renewable Energy, Sustainability and the Environment
- Fuel Technology
- Condensed Matter Physics
- Energy Engineering and Power Technology
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Development of solid oxide fuel cells (SOFCs) by tape-casting and single-step co-firing of monolithic laminates. / Myung, Jae Ha; Ko, Hyun Jun; Im, Chang Hyeok; Moon, Joo Ho; Hyun, Sang Hoon.
In: International Journal of Hydrogen Energy, Vol. 39, No. 5, 04.02.2014, p. 2313-2319.Research output: Contribution to journal › Article
TY - JOUR
T1 - Development of solid oxide fuel cells (SOFCs) by tape-casting and single-step co-firing of monolithic laminates
AU - Myung, Jae Ha
AU - Ko, Hyun Jun
AU - Im, Chang Hyeok
AU - Moon, Joo Ho
AU - Hyun, Sang Hoon
PY - 2014/2/4
Y1 - 2014/2/4
N2 - We developed a cost-effective method to manufacture high performance-monolithic solid oxide fuel cells using nano-composite electrodes, tape-casting and single-step co-firing. NiO/YSZ-YSZ nano-composite powder comprising nano-sized NiO and YSZ adhered to core YSZ powder was prepared for anode support. LSM/GDC nano-composite cathode fired at 1400 C had a porosity of over 20%, which was much higher than that of conventional LSM-GDC. Furthermore, the area specific resistance of the LSM/GDC cathode was 0.15 Ω cm 2, which was much lower than that of the LSM-GDC and LSM-YSZ mechanically mixed cathodes. Various types of monolithic SOFC unit cells were prepared; one consisting of a NiO-YSZ anode, NiO/YSZ-YSZ anode functional layer, and LSM-GDC cathode had a current density of 0.37 A/cm2 at 0.7 V at 800 C. Optimized monolithic SOFC consisting of NiO/YSZ-YSZ anode and YSZ electrolyte and LSM/GDC cathode had a greatly improved current density of 0.84 A/cm2.
AB - We developed a cost-effective method to manufacture high performance-monolithic solid oxide fuel cells using nano-composite electrodes, tape-casting and single-step co-firing. NiO/YSZ-YSZ nano-composite powder comprising nano-sized NiO and YSZ adhered to core YSZ powder was prepared for anode support. LSM/GDC nano-composite cathode fired at 1400 C had a porosity of over 20%, which was much higher than that of conventional LSM-GDC. Furthermore, the area specific resistance of the LSM/GDC cathode was 0.15 Ω cm 2, which was much lower than that of the LSM-GDC and LSM-YSZ mechanically mixed cathodes. Various types of monolithic SOFC unit cells were prepared; one consisting of a NiO-YSZ anode, NiO/YSZ-YSZ anode functional layer, and LSM-GDC cathode had a current density of 0.37 A/cm2 at 0.7 V at 800 C. Optimized monolithic SOFC consisting of NiO/YSZ-YSZ anode and YSZ electrolyte and LSM/GDC cathode had a greatly improved current density of 0.84 A/cm2.
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U2 - 10.1016/j.ijhydene.2013.11.122
DO - 10.1016/j.ijhydene.2013.11.122
M3 - Article
VL - 39
SP - 2313
EP - 2319
JO - International Journal of Hydrogen Energy
JF - International Journal of Hydrogen Energy
SN - 0360-3199
IS - 5
ER -