Extremely efficient flexible organic light-emitting diodes with modified graphene anode

Tae Hee Han, Youngbin Lee, Mi Ri Choi, Seong Hoon Woo, Sang Hoon Bae, Byung Hee Hong, Jong Hyun Ahn, Tae Woo Lee

Research output: Contribution to journalArticle

952 Citations (Scopus)

Abstract

Although graphene films have a strong potential to replace indium tin oxide anodes in organic light-emitting diodes (OLEDs), to date, the luminous efficiency of OLEDs with graphene anodes has been limited by a lack of efficient methods to improve the low work function and reduce the sheet resistance of graphene films to the levels required for electrodes1-4. Here, we fabricate flexible OLEDs by modifying the graphene anode to have a high work function and low sheet resistance, and thus achieve extremely high luminous efficiencies (37.2 lm W-1 in fluorescent OLEDs, 102.7 lm W -1 in phosphorescent OLEDs), which are significantly higher than those of optimized devices with an indium tin oxide anode (24.1 lm W -1 in fluorescent OLEDs, 85.6 lm W-1 in phosphorescent OLEDs). We also fabricate flexible white OLED lighting devices using the graphene anode. These results demonstrate the great potential of graphene anodes for use in a wide variety of high-performance flexible organic optoelectronics.

Original languageEnglish
Pages (from-to)105-110
Number of pages6
JournalNature Photonics
Volume6
Issue number2
DOIs
Publication statusPublished - 2012 Feb

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Graphite
Organic light emitting diodes (OLED)
Graphene
graphene
Anodes
anodes
light emitting diodes
Sheet resistance
Tin oxides
indium oxides
Indium
tin oxides
Optoelectronic devices
illuminating
Lighting

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Atomic and Molecular Physics, and Optics

Cite this

Han, T. H., Lee, Y., Choi, M. R., Woo, S. H., Bae, S. H., Hong, B. H., ... Lee, T. W. (2012). Extremely efficient flexible organic light-emitting diodes with modified graphene anode. Nature Photonics, 6(2), 105-110. https://doi.org/10.1038/nphoton.2011.318
Han, Tae Hee ; Lee, Youngbin ; Choi, Mi Ri ; Woo, Seong Hoon ; Bae, Sang Hoon ; Hong, Byung Hee ; Ahn, Jong Hyun ; Lee, Tae Woo. / Extremely efficient flexible organic light-emitting diodes with modified graphene anode. In: Nature Photonics. 2012 ; Vol. 6, No. 2. pp. 105-110.
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Han, TH, Lee, Y, Choi, MR, Woo, SH, Bae, SH, Hong, BH, Ahn, JH & Lee, TW 2012, 'Extremely efficient flexible organic light-emitting diodes with modified graphene anode', Nature Photonics, vol. 6, no. 2, pp. 105-110. https://doi.org/10.1038/nphoton.2011.318

Extremely efficient flexible organic light-emitting diodes with modified graphene anode. / Han, Tae Hee; Lee, Youngbin; Choi, Mi Ri; Woo, Seong Hoon; Bae, Sang Hoon; Hong, Byung Hee; Ahn, Jong Hyun; Lee, Tae Woo.

In: Nature Photonics, Vol. 6, No. 2, 02.2012, p. 105-110.

Research output: Contribution to journalArticle

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