Fabrication of stable electrospun TiO2 nanorods for high-performance dye-sensitized solar cells

Yeong Don Park, Keita Anabuki, Sumin Kim, Kyung Won Park, Dong Hyun Lee, Soong Ho Um, Jooyong Kim, Jeong Ho Cho

Research output: Contribution to journalArticle

13 Citations (Scopus)

Abstract

TiO2 multi-electrodes composed of nanoparticles and nanorods were prepared for use as electrodes in dye-sensitized solar cells (DSSC) in an effort to improve the light-to-electricity conversion efficiency. TiO 2 nanorods have been successfully prepared via electrospinning methods using a solution containing titanium isopropoxide (TIP). Acetic acid is generally used as a catalyst in sol-gel processes involving TIP; however, acetic acid induces rapid solidification of the sol solution, resulting in clogging of the nozzle during electrospinning, thereby hindering the mass production of TiO2 nanorods. In this work, we introduced acetyl acetone as a new catalyst and optimized the electrospinning conditions of TiO2 nanofibers. The use of acetyl acetone catalysts dramatically extended the solidification time of the TIP sol solution. The DSSC efficiency was improved through the use of TiO2 multi-electrodes. [Figure not available: see fulltext.]

Original languageEnglish
Pages (from-to)636-640
Number of pages5
JournalMacromolecular Research
Volume21
Issue number6
DOIs
Publication statusPublished - 2013 Jun 1

Fingerprint

Electrospinning
Nanorods
Titanium
Polymethyl Methacrylate
Sols
Acetone
Fabrication
Acetic acid
Acetic Acid
Electrodes
Catalysts
Rapid solidification
Nanofibers
Sol-gel process
Conversion efficiency
Solidification
Nozzles
Electricity
Nanoparticles
Dye-sensitized solar cells

All Science Journal Classification (ASJC) codes

  • Chemical Engineering(all)
  • Organic Chemistry
  • Polymers and Plastics
  • Materials Chemistry

Cite this

Park, Yeong Don ; Anabuki, Keita ; Kim, Sumin ; Park, Kyung Won ; Lee, Dong Hyun ; Um, Soong Ho ; Kim, Jooyong ; Cho, Jeong Ho. / Fabrication of stable electrospun TiO2 nanorods for high-performance dye-sensitized solar cells. In: Macromolecular Research. 2013 ; Vol. 21, No. 6. pp. 636-640.
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Fabrication of stable electrospun TiO2 nanorods for high-performance dye-sensitized solar cells. / Park, Yeong Don; Anabuki, Keita; Kim, Sumin; Park, Kyung Won; Lee, Dong Hyun; Um, Soong Ho; Kim, Jooyong; Cho, Jeong Ho.

In: Macromolecular Research, Vol. 21, No. 6, 01.06.2013, p. 636-640.

Research output: Contribution to journalArticle

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AU - Park, Yeong Don

AU - Anabuki, Keita

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AU - Lee, Dong Hyun

AU - Um, Soong Ho

AU - Kim, Jooyong

AU - Cho, Jeong Ho

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AB - TiO2 multi-electrodes composed of nanoparticles and nanorods were prepared for use as electrodes in dye-sensitized solar cells (DSSC) in an effort to improve the light-to-electricity conversion efficiency. TiO 2 nanorods have been successfully prepared via electrospinning methods using a solution containing titanium isopropoxide (TIP). Acetic acid is generally used as a catalyst in sol-gel processes involving TIP; however, acetic acid induces rapid solidification of the sol solution, resulting in clogging of the nozzle during electrospinning, thereby hindering the mass production of TiO2 nanorods. In this work, we introduced acetyl acetone as a new catalyst and optimized the electrospinning conditions of TiO2 nanofibers. The use of acetyl acetone catalysts dramatically extended the solidification time of the TIP sol solution. The DSSC efficiency was improved through the use of TiO2 multi-electrodes. [Figure not available: see fulltext.]

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