Facile synthesis of SnO 2 aerogel/reduced graphene oxide nanocomposites via in situ annealing for the photocatalytic degradation of methyl orange

Taehee Kim, Vinayak G. Parale, Hae Noo Ree Jung, Younghun Kim, Zied Driss, Dorra Driss, Abdallah Bouabidi, Souhir Euchy, Hyung Ho Park

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31 Citations (Scopus)

Abstract

SnO 2 aerogel/reduced graphene oxide (rGO) nanocomposites were synthesized using the sol–gel method. A homogeneous dispersion of graphene oxide (GO) flakes in a tin precursor solution was captured in a three-dimensional network SnO 2 aerogel matrix and successively underwent supercritical alcohol drying followed by the in situ thermal reduction of GO, resulting in SnO 2 aerogel/rGO nanocomposites. The chemical interaction between aerogel matrix and GO functional groups was confirmed by a peak shift in the Fourier transform infrared spectra and a change in the optical bandgap of the diffuse reflectance spectra. The role of rGO in 3D aerogel structure was studied in terms of photocatalytic activity with detailed mechanism of the enhancement such as electron transfer between the GO and SnO 2 . In addition, the photocatalytic activity of these nanocomposites in the methyl orange degradation varied depending on the amount of rGO loading in the SnO 2 aerogel matrix; an appropriate amount of rGO was required for the highest enhancement in the photocatalytic activity of the SnO 2 aerogel. The proposed nanocomposites could be a useful solution against water pollutants.

Original languageEnglish
Article number358
JournalNanomaterials
Volume9
Issue number3
DOIs
Publication statusPublished - 2019 Mar

Bibliographical note

Funding Information:
This work was supported by ‘Korea-Africa Joint Research Programme’ grant funded by the Korea government (Ministry of Science, Technology & ICT) in 2017K1A3A1A09085891. This work was supported (researched) by the third Stage of Brain Korea 21 Plus Project in 2019.

Publisher Copyright:
© 2019 by the authors. Licensee MDPI, Basel, Switzerland.

All Science Journal Classification (ASJC) codes

  • Chemical Engineering(all)
  • Materials Science(all)

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