Femtosecond free induction decay of metal surface adsorbate vibrations

J. C. Owrutsky, J. P. Culver, M. Li, Y. R. Kim, M. J. Sarsiky, M. S. Yeganeh, R. M. Hochstrasser, A. G. Yodh

Research output: Chapter in Book/Report/Conference proceedingChapter

1 Citation (Scopus)

Abstract

Recently there has been intense interest in the vibrational dynamics of molecular adsorbates on simple surfaces. In this contribution we present free induction decay (FID) measurements of the vibrational dephasing of CO adsorbed on Cu(111). To our knowledge this represents the first measurement of a FID signal from an adsorbate on a metal, and the fastest coherent transient IR measurement performed on surface adsorbates thus far. The experiments described are the first in a series of ultrafast surface dynamical studies that are underway in our laboratory.

Original languageEnglish
Title of host publicationUltrafast Phenomena VIII
PublisherPubl by Springer-Verlag GmbH & Company KG
Pages345-346
Number of pages2
Edition55
ISBN (Print)3540564756
Publication statusPublished - 1993 Jan 1
EventProceedings of the 8th International Conference on Ultrafast Phenomena - Antibes Juan-Les-Pins, France
Duration: 1992 Jun 81992 Jun 12

Other

OtherProceedings of the 8th International Conference on Ultrafast Phenomena
CityAntibes Juan-Les-Pins, France
Period92/6/892/6/12

Fingerprint

Adsorbates
metal surfaces
induction
Metals
vibration
decay
Carbon Monoxide
metals
Experiments

All Science Journal Classification (ASJC) codes

  • Physical and Theoretical Chemistry

Cite this

Owrutsky, J. C., Culver, J. P., Li, M., Kim, Y. R., Sarsiky, M. J., Yeganeh, M. S., ... Yodh, A. G. (1993). Femtosecond free induction decay of metal surface adsorbate vibrations. In Ultrafast Phenomena VIII (55 ed., pp. 345-346). Publ by Springer-Verlag GmbH & Company KG.
Owrutsky, J. C. ; Culver, J. P. ; Li, M. ; Kim, Y. R. ; Sarsiky, M. J. ; Yeganeh, M. S. ; Hochstrasser, R. M. ; Yodh, A. G. / Femtosecond free induction decay of metal surface adsorbate vibrations. Ultrafast Phenomena VIII. 55. ed. Publ by Springer-Verlag GmbH & Company KG, 1993. pp. 345-346
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Owrutsky, JC, Culver, JP, Li, M, Kim, YR, Sarsiky, MJ, Yeganeh, MS, Hochstrasser, RM & Yodh, AG 1993, Femtosecond free induction decay of metal surface adsorbate vibrations. in Ultrafast Phenomena VIII. 55 edn, Publ by Springer-Verlag GmbH & Company KG, pp. 345-346, Proceedings of the 8th International Conference on Ultrafast Phenomena, Antibes Juan-Les-Pins, France, 92/6/8.

Femtosecond free induction decay of metal surface adsorbate vibrations. / Owrutsky, J. C.; Culver, J. P.; Li, M.; Kim, Y. R.; Sarsiky, M. J.; Yeganeh, M. S.; Hochstrasser, R. M.; Yodh, A. G.

Ultrafast Phenomena VIII. 55. ed. Publ by Springer-Verlag GmbH & Company KG, 1993. p. 345-346.

Research output: Chapter in Book/Report/Conference proceedingChapter

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T1 - Femtosecond free induction decay of metal surface adsorbate vibrations

AU - Owrutsky, J. C.

AU - Culver, J. P.

AU - Li, M.

AU - Kim, Y. R.

AU - Sarsiky, M. J.

AU - Yeganeh, M. S.

AU - Hochstrasser, R. M.

AU - Yodh, A. G.

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N2 - Recently there has been intense interest in the vibrational dynamics of molecular adsorbates on simple surfaces. In this contribution we present free induction decay (FID) measurements of the vibrational dephasing of CO adsorbed on Cu(111). To our knowledge this represents the first measurement of a FID signal from an adsorbate on a metal, and the fastest coherent transient IR measurement performed on surface adsorbates thus far. The experiments described are the first in a series of ultrafast surface dynamical studies that are underway in our laboratory.

AB - Recently there has been intense interest in the vibrational dynamics of molecular adsorbates on simple surfaces. In this contribution we present free induction decay (FID) measurements of the vibrational dephasing of CO adsorbed on Cu(111). To our knowledge this represents the first measurement of a FID signal from an adsorbate on a metal, and the fastest coherent transient IR measurement performed on surface adsorbates thus far. The experiments described are the first in a series of ultrafast surface dynamical studies that are underway in our laboratory.

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Owrutsky JC, Culver JP, Li M, Kim YR, Sarsiky MJ, Yeganeh MS et al. Femtosecond free induction decay of metal surface adsorbate vibrations. In Ultrafast Phenomena VIII. 55 ed. Publ by Springer-Verlag GmbH & Company KG. 1993. p. 345-346