Femtosecond free induction decay of metal surface adsorbate vibrations

J. C. Owrutsky; J. P. Culver; M. Li; Y. R. Kim; M. J. Sarsiky; M. S. Yeganeh; R. M. Hochstrasser; A. G. Yodh

Femtosecond free induction decay of metal surface adsorbate vibrations

J. C. Owrutsky, J. P. Culver, M. Li, Y. R. Kim, M. J. Sarsiky, M. S. Yeganeh, R. M. Hochstrasser, A. G. Yodh

Department of Chemistry

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1 Citation (Scopus)

Abstract

Recently there has been intense interest in the vibrational dynamics of molecular adsorbates on simple surfaces. In this contribution we present free induction decay (FID) measurements of the vibrational dephasing of CO adsorbed on Cu(111). To our knowledge this represents the first measurement of a FID signal from an adsorbate on a metal, and the fastest coherent transient IR measurement performed on surface adsorbates thus far. The experiments described are the first in a series of ultrafast surface dynamical studies that are underway in our laboratory.

Original language	English
Title of host publication	Ultrafast Phenomena VIII
Publisher	Publ by Springer-Verlag GmbH & Company KG
Pages	345-346
Number of pages	2
Edition	55
ISBN (Print)	3540564756
Publication status	Published - 1993
Event	Proceedings of the 8th International Conference on Ultrafast Phenomena - Antibes Juan-Les-Pins, France Duration: 1992 Jun 8 → 1992 Jun 12

Other

Other	Proceedings of the 8th International Conference on Ultrafast Phenomena
City	Antibes Juan-Les-Pins, France
Period	92/6/8 → 92/6/12

All Science Journal Classification (ASJC) codes

Physical and Theoretical Chemistry

Cite this

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title = "Femtosecond free induction decay of metal surface adsorbate vibrations",

abstract = "Recently there has been intense interest in the vibrational dynamics of molecular adsorbates on simple surfaces. In this contribution we present free induction decay (FID) measurements of the vibrational dephasing of CO adsorbed on Cu(111). To our knowledge this represents the first measurement of a FID signal from an adsorbate on a metal, and the fastest coherent transient IR measurement performed on surface adsorbates thus far. The experiments described are the first in a series of ultrafast surface dynamical studies that are underway in our laboratory.",

author = "Owrutsky, {J. C.} and Culver, {J. P.} and M. Li and Kim, {Y. R.} and Sarsiky, {M. J.} and Yeganeh, {M. S.} and Hochstrasser, {R. M.} and Yodh, {A. G.}",

year = "1993",

language = "English",

isbn = "3540564756",

pages = "345--346",

booktitle = "Ultrafast Phenomena VIII",

publisher = "Publ by Springer-Verlag GmbH & Company KG",

edition = "55",

note = "Proceedings of the 8th International Conference on Ultrafast Phenomena ; Conference date: 08-06-1992 Through 12-06-1992",

}

Owrutsky, JC, Culver, JP, Li, M, Kim, YR, Sarsiky, MJ, Yeganeh, MS, Hochstrasser, RM & Yodh, AG 1993, Femtosecond free induction decay of metal surface adsorbate vibrations. in Ultrafast Phenomena VIII. 55 edn, Publ by Springer-Verlag GmbH & Company KG, pp. 345-346, Proceedings of the 8th International Conference on Ultrafast Phenomena, Antibes Juan-Les-Pins, France, 92/6/8.

TY - CHAP

T1 - Femtosecond free induction decay of metal surface adsorbate vibrations

AU - Owrutsky, J. C.

AU - Culver, J. P.

AU - Li, M.

AU - Kim, Y. R.

AU - Sarsiky, M. J.

AU - Yeganeh, M. S.

AU - Hochstrasser, R. M.

AU - Yodh, A. G.

PY - 1993

Y1 - 1993

N2 - Recently there has been intense interest in the vibrational dynamics of molecular adsorbates on simple surfaces. In this contribution we present free induction decay (FID) measurements of the vibrational dephasing of CO adsorbed on Cu(111). To our knowledge this represents the first measurement of a FID signal from an adsorbate on a metal, and the fastest coherent transient IR measurement performed on surface adsorbates thus far. The experiments described are the first in a series of ultrafast surface dynamical studies that are underway in our laboratory.

AB - Recently there has been intense interest in the vibrational dynamics of molecular adsorbates on simple surfaces. In this contribution we present free induction decay (FID) measurements of the vibrational dephasing of CO adsorbed on Cu(111). To our knowledge this represents the first measurement of a FID signal from an adsorbate on a metal, and the fastest coherent transient IR measurement performed on surface adsorbates thus far. The experiments described are the first in a series of ultrafast surface dynamical studies that are underway in our laboratory.

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M3 - Chapter

AN - SCOPUS:0027805214

SN - 3540564756

SP - 345

EP - 346

BT - Ultrafast Phenomena VIII

PB - Publ by Springer-Verlag GmbH & Company KG

T2 - Proceedings of the 8th International Conference on Ultrafast Phenomena

Y2 - 8 June 1992 through 12 June 1992

ER -

Femtosecond free induction decay of metal surface adsorbate vibrations

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