Formation and manipulation of confined water wires

Yongjae Lee, C. Dave Martin, John B. Parise, Joseph A. Hriljac, Thomas Vogt

Research output: Contribution to journalArticle

23 Citations (Scopus)

Abstract

Pressure-induced hydration (PIH) in the zeolite natrolite leads to well-ordered one-dimensional "water wires" and "water tubes". These structures provide urgently needed points of reference for molecular dynamics simulations and serve as models of transient and disordered biological nanowater. We show here that applying simultaneous pressure and temperature using a hydrothermal diamond anvil cell permits the intermolecular manipulation of water wires due to changes in the geometry of the host scaffolding and the enclosed hydrogen bonded water. During this process the ordered water wires formed under pressure change their direction depending on the temperature. This provides the opportunity to study the dynamics of confined water at the nanoscale by temperature and/or pressure-jump experiments. Our studies indicate that confined water responds differently to pressure and temperature than does bulk water.

Original languageEnglish
Pages (from-to)619-621
Number of pages3
JournalNano Letters
Volume4
Issue number4
DOIs
Publication statusPublished - 2004 Apr 1

Fingerprint

manipulators
wire
Wire
Water
water
Zeolites
Temperature
Diamond
temperature
anvils
Hydration
hydration
Molecular dynamics
Hydrogen
Diamonds
diamonds
molecular dynamics
tubes
Geometry
Computer simulation

All Science Journal Classification (ASJC) codes

  • Bioengineering
  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanical Engineering

Cite this

Lee, Y., Martin, C. D., Parise, J. B., Hriljac, J. A., & Vogt, T. (2004). Formation and manipulation of confined water wires. Nano Letters, 4(4), 619-621. https://doi.org/10.1021/nl049946n
Lee, Yongjae ; Martin, C. Dave ; Parise, John B. ; Hriljac, Joseph A. ; Vogt, Thomas. / Formation and manipulation of confined water wires. In: Nano Letters. 2004 ; Vol. 4, No. 4. pp. 619-621.
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Lee, Y, Martin, CD, Parise, JB, Hriljac, JA & Vogt, T 2004, 'Formation and manipulation of confined water wires', Nano Letters, vol. 4, no. 4, pp. 619-621. https://doi.org/10.1021/nl049946n

Formation and manipulation of confined water wires. / Lee, Yongjae; Martin, C. Dave; Parise, John B.; Hriljac, Joseph A.; Vogt, Thomas.

In: Nano Letters, Vol. 4, No. 4, 01.04.2004, p. 619-621.

Research output: Contribution to journalArticle

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Lee Y, Martin CD, Parise JB, Hriljac JA, Vogt T. Formation and manipulation of confined water wires. Nano Letters. 2004 Apr 1;4(4):619-621. https://doi.org/10.1021/nl049946n