Ion-Gel-Gated Graphene Optical Modulator with Hysteretic Behavior

Jin Tae Kim, Hongkyw Choi, Yongsuk Choi, Jeong Ho Cho

Research output: Contribution to journalArticle

13 Citations (Scopus)

Abstract

We propose a graphene-based optical modulator and comprehensively investigate its photonic characteristics by electrically controlling the device with an ion-gel top-gate dielectric. The density of the electrically driven charge carriers in the ion-gel gate dielectric plays a key role in tuning the optical output power of the device. The charge density at the ion-gel-graphene interface is tuned electrically, and the chemical potential of graphene is then changed to control its light absorption strength. The optical behavior of the ion-gel gate dielectric exhibits a large hysteresis which originates from the inherent nature of the ionic gel and the graphene-ion-gel interface and a slow polarization response time of ions. The photonic device is applicable to both TE- and TM-polarized light waves, covering two entire optical communication bands, the O-band (1.26-1.36 μm) and the C-band (1.52-1.565 μm). The experimental results are in good agreement with theoretically simulated predictions. The temporal behavior of the ion-gel-graphene-integrated optical modulator reveals a long-term modulation state because of the relatively low mobility of the ions in the ion-gel solution and formation of the electric double layer in the graphene-ion-gel interface. Fast dynamic recovery is observed by applying an opposite voltage gate pulse. This study paves the way to the understanding of the operational principles and future applications of ion-gel-gated graphene optical devices in photonics.

Original languageEnglish
Pages (from-to)1836-1845
Number of pages10
JournalACS Applied Materials and Interfaces
Volume10
Issue number2
DOIs
Publication statusPublished - 2018 Jan 17

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Light modulators
Graphene
Gels
Ions
Gate dielectrics
Photonics
Photonic devices
Chemical potential
Light polarization
Optical communication
Optical devices
Charge density
Charge carriers
Light absorption
Hysteresis
Tuning
Modulation
Polarization

All Science Journal Classification (ASJC) codes

  • Materials Science(all)

Cite this

Kim, Jin Tae ; Choi, Hongkyw ; Choi, Yongsuk ; Cho, Jeong Ho. / Ion-Gel-Gated Graphene Optical Modulator with Hysteretic Behavior. In: ACS Applied Materials and Interfaces. 2018 ; Vol. 10, No. 2. pp. 1836-1845.
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Ion-Gel-Gated Graphene Optical Modulator with Hysteretic Behavior. / Kim, Jin Tae; Choi, Hongkyw; Choi, Yongsuk; Cho, Jeong Ho.

In: ACS Applied Materials and Interfaces, Vol. 10, No. 2, 17.01.2018, p. 1836-1845.

Research output: Contribution to journalArticle

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