Lead-free halide double perovskites: Toward stable and sustainable optoelectronic devices

Asia Bibi, Ilgeum Lee, Yoonseo Nah, Omar Allam, Heejun Kim, Li Na Quan, Jiang Tang, Aron Walsh, Seung Soon Jang, Edward H. Sargent, Dong Ha Kim

Research output: Contribution to journalReview articlepeer-review

Abstract

In recent years, metal halide perovskites (MHPs) have attracted attention as semiconductors that achieve desirable properties for optoelectronic devices. However, two challenges—instability and the regulated nature of Pb —remain to be addressed with commercial applications. The development of Pb-free halide double perovskite (HDP) materials has gained interest and attention as a result. This family offers potential in the field of optoelectronic devices through flexible material designs and compositional adjustments. We highlight recent progress and development in halide double perovskites and encompass the synthesis, optoelectronic properties, and engineering of the electronic structures of these materials along with their applications in optoelectronic devices. Computational and data-driven statistical methods can also be used to explore mechanisms and discover promising candidate double perovskites.

Original languageEnglish
JournalMaterials Today
DOIs
Publication statusAccepted/In press - 2021

Bibliographical note

Funding Information:
This work was supported by National Research Foundation of Korea Grant funded by the Korean Government ( NRF-2020R 1A 2C 3003958 ), the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government (MOTIE) (No. 20173010013340 ) and Korea Basic Science Institute (National Research Facilities and Equipment Center) grant funded by the Ministry of Education ( 2020R 1A 6C 101B194 ). J. Tang acknowledged the financial support by the Major State Basic Research Development Program of China ( 2016YFB0700702 , 2018YFA0703200 ).

Publisher Copyright:
© 2020

All Science Journal Classification (ASJC) codes

  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering

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