Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles

Cuiling Li; Muhammad Iqbal; Bo Jiang; Zhongli Wang; Jeonghun Kim; Ashok Kumar Nanjundan; Andrew E. Whitten; Kathleen Wood; Yusuke Yamauchi

doi:10.1039/C8SC03911A

Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles

Cuiling Li, Muhammad Iqbal, Bo Jiang, Zhongli Wang, Jeonghun Kim, Ashok Kumar Nanjundan, Andrew E. Whitten, Kathleen Wood, Yusuke Yamauchi

Department of Chemical and Biomolecular Engineering

Research output: Contribution to journal › Article › peer-review

117 Citations (Scopus)

Abstract

Understanding how mesoporous noble metal architectures affect electrocatalytic performance is very important for the rational design and preparation of high-performance electrocatalysts. Herein, by using polymeric micelle-assembled structures as templates, mesoporous Pd nanoparticles with tunable porous constructions are synthesized by simply tuning the solvent compositions. The effect of porous Pd nanoparticles on the electrocatalytic performance is thoroughly studied. Their superior electrocatalytic activity can be attributed to the mass transport efficiency and open porous structures.

Original language	English
Pages (from-to)	4054-4061
Number of pages	8
Journal	Chemical Science
Volume	10
Issue number	14
DOIs	https://doi.org/10.1039/C8SC03911A
Publication status	Published - 2019 Apr 14

Bibliographical note

Funding Information:
This work was supported by the Australian Research Council (ARC) Future Fellow (grant FT150100479). The authors extend their appreciation to QUST for funding this research work. This work was performed in part at the Queensland node of the Australian National Fabrication Facility, a company established under the National Collaborative Research Infrastructure Strategy to provide nano-and micro-fabrication facilities for Australia's researchers.

Publisher Copyright:
© The Royal Society of Chemistry.

All Science Journal Classification (ASJC) codes

Chemistry(all)

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10.1039/C8SC03911A

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abstract = "Understanding how mesoporous noble metal architectures affect electrocatalytic performance is very important for the rational design and preparation of high-performance electrocatalysts. Herein, by using polymeric micelle-assembled structures as templates, mesoporous Pd nanoparticles with tunable porous constructions are synthesized by simply tuning the solvent compositions. The effect of porous Pd nanoparticles on the electrocatalytic performance is thoroughly studied. Their superior electrocatalytic activity can be attributed to the mass transport efficiency and open porous structures.",

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Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles. / Li, Cuiling; Iqbal, Muhammad; Jiang, Bo; Wang, Zhongli; Kim, Jeonghun; Nanjundan, Ashok Kumar; Whitten, Andrew E.; Wood, Kathleen; Yamauchi, Yusuke.

In: Chemical Science, Vol. 10, No. 14, 14.04.2019, p. 4054-4061.

Research output: Contribution to journal › Article › peer-review

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AU - Nanjundan, Ashok Kumar

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AU - Wood, Kathleen

AU - Yamauchi, Yusuke

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Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles

Abstract

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