Redshift of the excited state due to a nondegenerate biexciton in self-organized quantum dots

K. Kim, T. B. Norris, U. Hohenester

Research output: Contribution to journalArticle

3 Citations (Scopus)

Abstract

Using femtosecond differential transmission spectroscopy, we observed a "nondegenerate" biexciton, consisting of an electron-hole pair in the dot ground state and an electron-hole pair in the excited state, in InGaAs self-organized quantum dots. We resonantly pumped the ground state transition in the quantum dots and observed an induced resonance in the probe differential transmission spectrum near the first excited-state transition, which we attribute to the formation of a nondegenerate biexciton state. The binding energy of 15 meV does not change with excitation power, thus reflecting a genuine feature of few-particle states. Our theoretical model calculations show good agreement with these experimental results. When a prepulse is used to generate a population inversion in the quantum dots, we also observed the effects of nondegenerate biexcitonic correlations in differential transmission.

Original languageEnglish
Article number113702
JournalJournal of Applied Physics
Volume103
Issue number11
DOIs
Publication statusPublished - 2008 Jun 20

Fingerprint

quantum dots
excitation
ground state
population inversion
binding energy
probes
spectroscopy

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy(all)

Cite this

@article{19016fdf978f43a790e5affc8142a0ca,
title = "Redshift of the excited state due to a nondegenerate biexciton in self-organized quantum dots",
abstract = "Using femtosecond differential transmission spectroscopy, we observed a {"}nondegenerate{"} biexciton, consisting of an electron-hole pair in the dot ground state and an electron-hole pair in the excited state, in InGaAs self-organized quantum dots. We resonantly pumped the ground state transition in the quantum dots and observed an induced resonance in the probe differential transmission spectrum near the first excited-state transition, which we attribute to the formation of a nondegenerate biexciton state. The binding energy of 15 meV does not change with excitation power, thus reflecting a genuine feature of few-particle states. Our theoretical model calculations show good agreement with these experimental results. When a prepulse is used to generate a population inversion in the quantum dots, we also observed the effects of nondegenerate biexcitonic correlations in differential transmission.",
author = "K. Kim and Norris, {T. B.} and U. Hohenester",
year = "2008",
month = "6",
day = "20",
doi = "10.1063/1.2913496",
language = "English",
volume = "103",
journal = "Journal of Applied Physics",
issn = "0021-8979",
publisher = "American Institute of Physics Publising LLC",
number = "11",

}

Redshift of the excited state due to a nondegenerate biexciton in self-organized quantum dots. / Kim, K.; Norris, T. B.; Hohenester, U.

In: Journal of Applied Physics, Vol. 103, No. 11, 113702, 20.06.2008.

Research output: Contribution to journalArticle

TY - JOUR

T1 - Redshift of the excited state due to a nondegenerate biexciton in self-organized quantum dots

AU - Kim, K.

AU - Norris, T. B.

AU - Hohenester, U.

PY - 2008/6/20

Y1 - 2008/6/20

N2 - Using femtosecond differential transmission spectroscopy, we observed a "nondegenerate" biexciton, consisting of an electron-hole pair in the dot ground state and an electron-hole pair in the excited state, in InGaAs self-organized quantum dots. We resonantly pumped the ground state transition in the quantum dots and observed an induced resonance in the probe differential transmission spectrum near the first excited-state transition, which we attribute to the formation of a nondegenerate biexciton state. The binding energy of 15 meV does not change with excitation power, thus reflecting a genuine feature of few-particle states. Our theoretical model calculations show good agreement with these experimental results. When a prepulse is used to generate a population inversion in the quantum dots, we also observed the effects of nondegenerate biexcitonic correlations in differential transmission.

AB - Using femtosecond differential transmission spectroscopy, we observed a "nondegenerate" biexciton, consisting of an electron-hole pair in the dot ground state and an electron-hole pair in the excited state, in InGaAs self-organized quantum dots. We resonantly pumped the ground state transition in the quantum dots and observed an induced resonance in the probe differential transmission spectrum near the first excited-state transition, which we attribute to the formation of a nondegenerate biexciton state. The binding energy of 15 meV does not change with excitation power, thus reflecting a genuine feature of few-particle states. Our theoretical model calculations show good agreement with these experimental results. When a prepulse is used to generate a population inversion in the quantum dots, we also observed the effects of nondegenerate biexcitonic correlations in differential transmission.

UR - http://www.scopus.com/inward/record.url?scp=45149099615&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=45149099615&partnerID=8YFLogxK

U2 - 10.1063/1.2913496

DO - 10.1063/1.2913496

M3 - Article

AN - SCOPUS:45149099615

VL - 103

JO - Journal of Applied Physics

JF - Journal of Applied Physics

SN - 0021-8979

IS - 11

M1 - 113702

ER -