Selective Light-Induced Patterning of Carbon Nanotube/Silver Nanoparticle Composite to Produce Extremely Flexible Conductive Electrodes

Inhyuk Kim, Kyoohee Woo, Zhaoyang Zhong, Eonseok Lee, Dongwoo Kang, Sunho Jeong, Young Man Choi, Yunseok Jang, Sin Kwon, Jooho Moon

Research output: Contribution to journalArticlepeer-review

40 Citations (Scopus)


Recently, highly flexible conductive features have been widely demanded for the development of various electronic applications, such as foldable displays, deformable lighting, disposable sensors, and flexible batteries. Herein, we report for the first time a selective photonic sintering-derived, highly reliable patterning approach for creating extremely flexible carbon nanotube (CNT)/silver nanoparticle (Ag NP) composite electrodes that can tolerate severe bending (20 000 cycles at a bending radius of 1 mm). The incorporation of CNTs into a Ag NP film can enhance not only the mechanical stability of electrodes but also the photonic-sintering efficiency when the composite is irradiated by intense pulsed light (IPL). Composite electrodes were patterned on various plastic substrates by a three-step process comprising coating, selective IPL irradiation, and wiping. A composite film selectively exposed to IPL could not be easily wiped from the substrate, because interfusion induced strong adhesion to the underlying polymer substrate. In contrast, a nonirradiated film adhered weakly to the substrate and was easily removed, enabling highly flexible patterned electrodes. The potential of our flexible electrode patterns was clearly demonstrated by fabricating a light-emitting diode circuit and a flexible transparent heater with unimpaired functionality under bending, rolling, and folding.

Original languageEnglish
Pages (from-to)6163-6170
Number of pages8
JournalACS Applied Materials and Interfaces
Issue number7
Publication statusPublished - 2017 Feb 22

Bibliographical note

Funding Information:
This work was supported by the Ministry of Trade, Industry & Energy (MOTIE Korea) under Advanced Technology Center (ATC) Program (10067668) and Technology Innovation Program (10052802). It was also supported by a National Research Foundation of Korea (NRF) funded by the Korean government (MSIP) (2012R1A3A2026417).

Publisher Copyright:
© 2017 American Chemical Society.

All Science Journal Classification (ASJC) codes

  • Materials Science(all)


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