Solution-deposited Zr-doped AlOx gate dielectrics enabling high-performance flexible transparent thin film transistors

Wooseok Yang, Keunkyu Song, Yangho Jung, Sunho Jeong, Jooho Moon

Research output: Contribution to journalArticle

99 Citations (Scopus)

Abstract

Although high dielectric constant (k) oxide thin film has been considered as a key element for high performance and low-voltage driven thin-film transistors (TFTs), there are no solution processable high-k oxide dielectrics that satisfy the stringent requirements of low-temperature processability, mechanical flexibility, and good TFT performance. Here, we demonstrate that the incorporation of a zirconium component that has strong bonding to oxygen enables a significant reduction in the processing temperature for soluble alumina dielectrics to as low as 250 °C. Based on these Zr-AlOx films, high performance, low operational voltage, flexible TFTs are achieved. Flexible TFTs operate well under a gate bias of 5 V, exhibiting a high saturation mobility of 51 cm2 V-1 s-1, an on/off current ratio of 104, and a low threshold voltage of 1.2 V with good mechanical flexibility. This is the first study demonstrating the mechanical flexibility of all-oxide soluble high-k dielectric-semiconductor-based TFTs with an emphasis on the influence of annealing temperature on the solution-deposited high-k oxide dielectric characteristics.

Original languageEnglish
Pages (from-to)4275-4282
Number of pages8
JournalJournal of Materials Chemistry C
Volume1
Issue number27
DOIs
Publication statusPublished - 2013 Jul 21

All Science Journal Classification (ASJC) codes

  • Chemistry(all)
  • Materials Chemistry

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