Synthesis of reduced graphene oxide/aluminum nanocomposites via chemical-mechanical processes

Daeyoung Kim, Heon Kang, Donghyun Bae, Seungjin Nam, Manuel Quevedo-Lopez, Hyunjoo Choi

Research output: Contribution to journalArticlepeer-review

Abstract

The present study employed a combination of solution-based synthesis and mechanical milling to develop reduced graphene oxide/aluminum composites, in order to achieve uniform dispersion of reduced graphene oxide and strong interfaces between reduced graphene oxide and aluminum. First, spherical aluminum powder was flattened via mechanical milling to afford a large specific surface area and many reaction sites for the graphene oxide. A hydrophilic surface was then created by coating the aluminum powder with polyvinyl alcohol. The polyvinyl alcohol-coated aluminum slurry was mixed with a graphene oxide suspension, thereby inducing a reaction between graphene oxide and polyvinyl alcohol via hydrogen bonding. After thermal reduction, the composite powder was further ball milled and hot-pressed at 500℃ to produce a reduced graphene oxide/aluminum composite. The dispersion of reduced graphene oxide in the composite, as well as the mechanical and thermal behaviors of the composite, improved with increased flattening and specific surface area of the starting aluminum powder.

Original languageEnglish
Pages (from-to)3015-3025
Number of pages11
JournalJournal of Composite Materials
Volume52
Issue number22
DOIs
Publication statusPublished - 2018 Sep 1

Bibliographical note

Funding Information:
The author(s) disclosed receipt of the following financial support for the research, authorship, and/or publication of this article: This work was supported by the Leading Foreign Research Institute Recruitment Program through the NRF funded by the Ministry of Science, ICT, & Future Planning (MSIP) (2013K1A4A3055679). H. Choi acknowledges the support from the Basic Science Research Program (2015R1D1A1A01060718, 2016M2B2A9A02943809, and 2017M1A3A3A02015639) through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science, and Technology.

All Science Journal Classification (ASJC) codes

  • Ceramics and Composites
  • Mechanics of Materials
  • Mechanical Engineering
  • Materials Chemistry

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