The effect of preparation method on the catalytic performance over superior MgO-promoted Ni-Ce0.8Zr0.2O2 catalyst for CO2 reforming of CH4

Dae Woon Jeong; Won Jun Jang; Jae Oh Shim; Hyun Seog Roh; In Hyuk Son; Seung Jae Lee

doi:10.1016/j.ijhydene.2013.08.026

The effect of preparation method on the catalytic performance over superior MgO-promoted Ni-Ce_0.8Zr_0.2O₂ catalyst for CO₂ reforming of CH₄

Dae Woon Jeong, Won Jun Jang, Jae Oh Shim, Hyun Seog Roh, In Hyuk Son, Seung Jae Lee

Division of Environmental Engineering

Research output: Contribution to journal › Article › peer-review

42 Citations (Scopus)

Abstract

The effect of preparation method on MgO-promoted Ni-Ce_0.8Zr _0.2O₂ catalysts was investigated in CO₂ reforming of CH₄. Co-precipitated Ni-MgO-Ce_0.8Zr _0.2O₂ exhibited very high activity as well as stability (X_CH4 > 95% at 800 C for 200 h) due to high surface area, high dispersion of Ni, small Ni crystallite size, and easier reducibility. Four elements (Ni, Mg, Ce, and Zr) are located at the same position for the co-precipitated catalyst, resulting in easier reducibility.

Original language	English
Pages (from-to)	13649-13654
Number of pages	6
Journal	International Journal of Hydrogen Energy
Volume	38
Issue number	31
DOIs	https://doi.org/10.1016/j.ijhydene.2013.08.026
Publication status	Published - 2013 Oct 17

Bibliographical note

Funding Information:
This research was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Science , ICT and Future Planning ( 2013R1A1A1A05007370 ).

All Science Journal Classification (ASJC) codes

Renewable Energy, Sustainability and the Environment
Fuel Technology
Condensed Matter Physics
Energy Engineering and Power Technology

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title = "The effect of preparation method on the catalytic performance over superior MgO-promoted Ni-Ce0.8Zr0.2O2 catalyst for CO2 reforming of CH4",

abstract = "The effect of preparation method on MgO-promoted Ni-Ce0.8Zr 0.2O2 catalysts was investigated in CO2 reforming of CH4. Co-precipitated Ni-MgO-Ce0.8Zr 0.2O2 exhibited very high activity as well as stability (XCH4 > 95% at 800 C for 200 h) due to high surface area, high dispersion of Ni, small Ni crystallite size, and easier reducibility. Four elements (Ni, Mg, Ce, and Zr) are located at the same position for the co-precipitated catalyst, resulting in easier reducibility.",

author = "Jeong, {Dae Woon} and Jang, {Won Jun} and Shim, {Jae Oh} and Roh, {Hyun Seog} and Son, {In Hyuk} and Lee, {Seung Jae}",

note = "Funding Information: This research was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Science , ICT and Future Planning ( 2013R1A1A1A05007370 ). ",

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The effect of preparation method on the catalytic performance over superior MgO-promoted Ni-Ce_0.8Zr_0.2O₂ catalyst for CO₂ reforming of CH₄. / Jeong, Dae Woon; Jang, Won Jun; Shim, Jae Oh; Roh, Hyun Seog; Son, In Hyuk; Lee, Seung Jae.

In: International Journal of Hydrogen Energy, Vol. 38, No. 31, 17.10.2013, p. 13649-13654.

Research output: Contribution to journal › Article › peer-review

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AU - Shim, Jae Oh

AU - Roh, Hyun Seog

AU - Son, In Hyuk

AU - Lee, Seung Jae

N1 - Funding Information: This research was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Science , ICT and Future Planning ( 2013R1A1A1A05007370 ).

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AB - The effect of preparation method on MgO-promoted Ni-Ce0.8Zr 0.2O2 catalysts was investigated in CO2 reforming of CH4. Co-precipitated Ni-MgO-Ce0.8Zr 0.2O2 exhibited very high activity as well as stability (XCH4 > 95% at 800 C for 200 h) due to high surface area, high dispersion of Ni, small Ni crystallite size, and easier reducibility. Four elements (Ni, Mg, Ce, and Zr) are located at the same position for the co-precipitated catalyst, resulting in easier reducibility.

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