Ultrafast spin-state conversion in solvated transition metal complexes probed with femtosecond soft X-ray spectroscopy

Nils Huse, Hana Cho, Tae Kyu Kim, Lindsey Jamula, James K. McCusker, Frank M.F.de Groot, Robert W. Schoenlein

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Abstract

We report the first femtosecond soft x-ray spectroscopy of solvated transition-metal complexes: Structural dynamics mediate ultrafast spin-state conversion and symmetry-specific valence-charge localization. This study demonstrates the unique potential of ultrafast soft x-ray spectroscopy in solutions.

Original languageEnglish
Title of host publicationInternational Conference on Ultrafast Phenomena, UP 2010
Publication statusPublished - 2010 Dec 1
EventInternational Conference on Ultrafast Phenomena, UP 2010 - Snowmass Village, CO, United States
Duration: 2010 Jul 182010 Jul 23

Publication series

NameOptics InfoBase Conference Papers
ISSN (Electronic)2162-2701

Other

OtherInternational Conference on Ultrafast Phenomena, UP 2010
CountryUnited States
CitySnowmass Village, CO
Period10/7/1810/7/23

Fingerprint

Metal complexes
X ray spectroscopy
x ray spectroscopy
Transition metals
transition metals
Spectroscopy
X rays
dynamic structural analysis
Structural dynamics
spectroscopy
x rays
valence
symmetry

All Science Journal Classification (ASJC) codes

  • Instrumentation
  • Atomic and Molecular Physics, and Optics

Cite this

Huse, N., Cho, H., Kim, T. K., Jamula, L., McCusker, J. K., Groot, F. M. F. D., & Schoenlein, R. W. (2010). Ultrafast spin-state conversion in solvated transition metal complexes probed with femtosecond soft X-ray spectroscopy. In International Conference on Ultrafast Phenomena, UP 2010 (Optics InfoBase Conference Papers).
Huse, Nils ; Cho, Hana ; Kim, Tae Kyu ; Jamula, Lindsey ; McCusker, James K. ; Groot, Frank M.F.de ; Schoenlein, Robert W. / Ultrafast spin-state conversion in solvated transition metal complexes probed with femtosecond soft X-ray spectroscopy. International Conference on Ultrafast Phenomena, UP 2010. 2010. (Optics InfoBase Conference Papers).
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abstract = "We report the first femtosecond soft x-ray spectroscopy of solvated transition-metal complexes: Structural dynamics mediate ultrafast spin-state conversion and symmetry-specific valence-charge localization. This study demonstrates the unique potential of ultrafast soft x-ray spectroscopy in solutions.",
author = "Nils Huse and Hana Cho and Kim, {Tae Kyu} and Lindsey Jamula and McCusker, {James K.} and Groot, {Frank M.F.de} and Schoenlein, {Robert W.}",
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Huse, N, Cho, H, Kim, TK, Jamula, L, McCusker, JK, Groot, FMFD & Schoenlein, RW 2010, Ultrafast spin-state conversion in solvated transition metal complexes probed with femtosecond soft X-ray spectroscopy. in International Conference on Ultrafast Phenomena, UP 2010. Optics InfoBase Conference Papers, International Conference on Ultrafast Phenomena, UP 2010, Snowmass Village, CO, United States, 10/7/18.

Ultrafast spin-state conversion in solvated transition metal complexes probed with femtosecond soft X-ray spectroscopy. / Huse, Nils; Cho, Hana; Kim, Tae Kyu; Jamula, Lindsey; McCusker, James K.; Groot, Frank M.F.de; Schoenlein, Robert W.

International Conference on Ultrafast Phenomena, UP 2010. 2010. (Optics InfoBase Conference Papers).

Research output: Chapter in Book/Report/Conference proceedingConference contribution

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AU - Huse, Nils

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AU - Kim, Tae Kyu

AU - Jamula, Lindsey

AU - McCusker, James K.

AU - Groot, Frank M.F.de

AU - Schoenlein, Robert W.

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Huse N, Cho H, Kim TK, Jamula L, McCusker JK, Groot FMFD et al. Ultrafast spin-state conversion in solvated transition metal complexes probed with femtosecond soft X-ray spectroscopy. In International Conference on Ultrafast Phenomena, UP 2010. 2010. (Optics InfoBase Conference Papers).